NIMTE OpenIR  > 2018专题
Hybrid-State Dynamics of Dye Molecules and Surface Plasmon Polaritons under Ultrastrong Coupling Regime
Wang, Hai; Wang, Hai-Yu; Chen, Qi-Dai; Xu, Huai-Liang; Sun, Hong-Bo; Huang, Fangcheng; Raja, Waseem; Toma, Andrea; Zaccaria, Remo Proietti
2018
发表期刊LASER & PHOTONICS REVIEWS
卷号12期号:3
摘要The achievement of an ultrastrong coupling regime between surface plasmon modes generated by gold conical pits arrays and excitons associated to squaraine dye is demonstrated. Numerical and experimental steady-state reflection measurements demonstrate a remarkable Rabi splitting of 860 meV, to date the largest reported value involving surface plasmon modes. Furthermore, the dynamics of the hybrid states under the ultrastrong coupling regime is investigated by transient absorption spectroscopy. The results show that the upper bands are too short-lived to be detected, while the lower bands have a relatively shorter lifetime with respect to the bleaching recovery of pure squaraine dye. This result contradicts the behaviour of systems in strong coupling regimes, suggesting a different photophysics between strong and ultrastrong coupled systems.
关键词Light-matter Interaction Metallic Nanostructures Temperature Microcavity Excitons Arrays
学科领域Chemistry ; Science & Technology - Other Topics ; Materials Science
语种英语
文献类型期刊论文
条目标识符http://ir.nimte.ac.cn/handle/174433/16773
专题2018专题
推荐引用方式
GB/T 7714
Wang, Hai,Wang, Hai-Yu,Chen, Qi-Dai,et al. Hybrid-State Dynamics of Dye Molecules and Surface Plasmon Polaritons under Ultrastrong Coupling Regime[J]. LASER & PHOTONICS REVIEWS,2018,12(3).
APA Wang, Hai.,Wang, Hai-Yu.,Chen, Qi-Dai.,Xu, Huai-Liang.,Sun, Hong-Bo.,...&Zaccaria, Remo Proietti.(2018).Hybrid-State Dynamics of Dye Molecules and Surface Plasmon Polaritons under Ultrastrong Coupling Regime.LASER & PHOTONICS REVIEWS,12(3).
MLA Wang, Hai,et al."Hybrid-State Dynamics of Dye Molecules and Surface Plasmon Polaritons under Ultrastrong Coupling Regime".LASER & PHOTONICS REVIEWS 12.3(2018).
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