NIMTE OpenIR  > 2018专题
Further enhancement of the light-regulated mixed-potential signal with ZnO-based electrodes
Jin, Han; Zhang, Xiaowei; Hua, Changzhou; Zhang, Xin; Zou, Jie; Shen, Wenfeng; Jian, Jiawen
2018
发表期刊SENSORS AND ACTUATORS B-CHEMICAL
卷号255页码:3516-3522
摘要UV illumination has been confirmed to be essentially increased the response magnitude of potentiometric gas sensors. Nevertheless, the detection limit of the sensor is still inadequate for real application even upon UV light, whilst, how to efficiently enhance the light-regulated mixed-potential signal is still unclear. In this research, the strategy of using the more photoactive ZnO-based composite as the sensing electrode (SE) for potentially further enhancing the sensing value is proposed and confirmed. Typically, in comparison with ZnO-SE, ZnO-based composite SE is beneficial for further promoting the light-regulation effect. Particularly, when upon illumination, the detection limit of the sensor consisting of the composite electrode (towards benzene) reaches 0.109 ppm, while that of the value for the sensor using ZnO-SE is 0.898 ppm. The promoting mechanism is clarified from the perspective of the electrocatalytic activity & gas-phase reactivity. In summary, forming the ZnO-based composites makes them ideal for generating abundant e(-) and h(+) when upon illumination, leading to the obvious increase in the catalytic activity of both cathodic & anodic reaction and thereby further raised the mixed-potential signal. Conclusively, this proof-of-concept opens a brighter future for designing future high-performance potentiometric gas sensors. (C) 2017 Elsevier B.V. All rights reserved.
关键词Volatile Organic-compounds Ysz-based Sensor Sensing-electrode Gas Sensor Ppb Level Zno/in2o3 Heteronanostructures Monitoring Applications No2 Sensor Benzene Toluene
学科领域Materials Science
语种英语
文献类型期刊论文
条目标识符http://ir.nimte.ac.cn/handle/174433/16852
专题2018专题
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GB/T 7714
Jin, Han,Zhang, Xiaowei,Hua, Changzhou,et al. Further enhancement of the light-regulated mixed-potential signal with ZnO-based electrodes[J]. SENSORS AND ACTUATORS B-CHEMICAL,2018,255:3516-3522.
APA Jin, Han.,Zhang, Xiaowei.,Hua, Changzhou.,Zhang, Xin.,Zou, Jie.,...&Jian, Jiawen.(2018).Further enhancement of the light-regulated mixed-potential signal with ZnO-based electrodes.SENSORS AND ACTUATORS B-CHEMICAL,255,3516-3522.
MLA Jin, Han,et al."Further enhancement of the light-regulated mixed-potential signal with ZnO-based electrodes".SENSORS AND ACTUATORS B-CHEMICAL 255(2018):3516-3522.
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